From the ASP.NET background, I can say the TreeView Control usually works nice with XML, tabular or Relational data, But it is always very good with XML.
So, it's better to write your data in XML format and then bind it with the tree.
Or if you want, you can do the data binding through wizard also. In that case you will find new data source and that will lead you to either Sitemap or XmlDatsource.
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